Yes, that's the 1861 census we have for William Sr. and Mary Ann (Rider) Pulleyblank.
Here's what else I have on him.
In 1869, Mary Ann (Rider) dies.
In 1871, William Pulleyblank (sr.) was recorded as a Farm Servant with the Luscombe family in Balterscombe, Ugborough, Devon, England.
In 1881, William Pulleyblank (sr.) was recorded as an Ag Labourer living with his brother George at Aldsworth Hill, Westbourne, Sussex, England --this is near Chichester, the birthplace in question of my great great great grandpa William Thomas Pulleyblank b.1861
In April 1881 William Pulleyblank marries Mary Anne Oakley at Westbourne, Sussex, England.
In 1891, he was recorded as an Agricultural Labourer with his wife Mary A, a cook, in the Anna L Pearse home at Little Hilliers, Stopham, Sussex, England.
In 1901, he was recorded as a Jobbing Gardener, with his wife Mary Ann, a domestic cook, boarding with Anna L Pearse at Station Road, Wavendon, Buckinghamshire,
England. --a few miles from the Woburn Abbey
In 1911, he was as a Jobbing gardener, with his wife Mary Ann at Alms Houses, Woburn Sands, Buckinghamshire, England. --still close by to the Woburn Abbey
It sparks my interest that he moved all the way from North Huish/Plymouth area to the Chichester area, then to the Woburn area....